Kagakagari has taken a plane full of people hostage and offers to exchange their lives for the Igniter. However, the exchange soon turns violent putting the lives of the hostages at risk. Tomo must then attempt a very dangerous plan using Kurogane in order to save everyone that he cares about, but will it be enough?

Now that Kurogane has absorbed the stabiliser, people can see Misao, but Tomo is worried that she won't be able to hide her incorporeal nature from those around her. Meanwhile, Haruna and Susugihara explore a strange set of ruins in search of the Caster Machina. These recent events prompt the group to look back on the tragic plane crash which started them in motion, not only for Misao and Tomo, but for Shuri and Susugihara as well.

Following a mishap with some industrial strength glue whilst practicing for the three-legged race, Tomo and Takatsuki end up stuck together for the rest of the day. As if protecting each other's modesty and organising sleeping arrangements weren't trouble enough, Takatsuki's family is currently under threat from a rival group of demons who are out to assassinate them.

Tomo and the others are apparently saved by Tomo's brother, Naotaka and then taken in by Kagakagari and Kristina. Kagakagari reveals that the ruins are the remnants of an Asura Machina testing ground and that they may contain a way to free Burial Dolls like Kotori and Misao. However, before they can retrieve the device Kyomu arrives and tries to use Ania as a hostage.

Tomo, Takatsuki, Misao, An and Higuchi are all enjoying a working vacation at the beach but it isn't long before Tomo manages to upset Misao. Meanwhile, Shuri and Ania are investigating the ruins on a nearby island. However, it seems that Kagakagari and Kristina are also interested in them, as is Kyomu Satomi and the First Student Council.

Tomo is growing increasingly concerned about Misao and asks Shuri and Touru to locate his brother, Naotaka. In exchange Tomo must persuade the reclusive Science Club president Tokiya Kagayaki to return to school. However, this is not as easy as it first sounds so Tomo takes Misao and Takatsuki along to help. Tomo also learns that Touru and Tokiya have a very tragic connection to Kurogane.

While, Shuri and Reishirou are enjoying their Second Year trip to Hawaii, Tomo accidentally stumbles across a Plug-In for the Asura Machina. However, Kagakagari also wants the device and he attacks Tomo and the others in order to retrieve it. As such Tomo is forced to break his promise to Takatsuki and use Kurogane to fend him off.

Tomoharu Natsume survived a horrible plane crash but Misao, his close friend, did not and became a ghost that continued to be attached to him. Three years later, he moved out to a place rented by his brother to live on his own and attend Raku High since his mother remarried. On his first day in his new house, a mysterious girl called Shuri turns up and gives him a silver briefcase to look after on behalf of his brother who lives abroad. Soon after, Tomoharu and his best friend, a ghost named Misao Minakami, are attacked by various factions who all seek the 'Asura Machina' and 'Extractor'.

Whilst being forced to clean the school pool Tomo and the rest of the Science Club stumble across an underground cavern which leads them to the Rakuroa Ruins. Here Tomo sees a strange vision of an alternate world. However, before he can learn more the group is attacked by Castas Machina guarding the ruins and Touru has to show up to save them.

The Second years are preparing for a class trip to Hawaii. Meanwhile, Tomo and Misao attend a party hosted by Reishirou in memory of the anniversary of Aine's death. The party also features a very unusual performance competition in which everyone from Rikka to Takatsuki takes part and which Tomo and Misao end up winning.

With Ania kidnapped by Takaya Kagakagari Tomo, Shuri, Misao and Takatsuki race to save her. Meanwhile Ania learns that Kagakagari plans to sacrifice all the demons in the city in order to lift the curse of the Asura Machina. By the time Tomo and the others arrive the ceremony has already begun and they must work quickly in order to save both Ania and Takatsuki.

After receiving a cryptic warning from his brother, Tomo and the others come under attack from a mysterious woman and are forced into a trap set by Hiwako Torishima. The group are then saved by a powerful Asura Machina and Tomo makes a serious of shocking discovery's about his brother, Misao and the Asura Machina themselves.

Following Hagane's attack Tomo awakes to find himself all alone in the First World with no idea of how to get back. He soon encounters the 'Witch of Rakurowa High School', a strange Daughter and very strange versions of the people he knows. However, after a chance encounter with Tokiya's sister Aki he is reunited with Takatsuki. He also learns more about the Superstring Gravity Reactor accident that started everything.

Having been reunited with Ania, Tomo learns more about the effects that the Superstring Gravity Reactor accident is having on the First World and Ania's involvement with it. Later when a large group of Daughters attacks the school Aki and Ania are forced to use their demonic powers to protect those they care about and Tomo learns that in this world he has powers of his own.

Now back in the Second World Tomo and the others discover that they have 10 days until Tokiya can set his plan in motion. Tomo also discovers that he has inadvertently entered a contract with Takatsuki and that they now have a Daughter, Persephone. As if that wasn't enough Tomo is then appointed as the new President of the Third Student Council. Unfortunately, there is no time to deal with all of these new events as Tokiya has a found a way to accelerate his plan and Tomo must once again try to save the world.

With a large creature mysteriously attacking demons, Takatsuki is forced by her family to move in with Tomo so that he can protect her. At the same time Shuri arrives with a young demon named Ania, who Tomo also has to protect. However, Ania is a 'Luck-Eater' and causes misfortune to befall Tomo and his friends. Things get even more complicated when it turns out that Ania's sister, Kristina maybe involved with the demon hunts.